Read-Out and Coherent Manipulation of an Isolated Nuclear Spin

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The thesis explores groundbreaking advancements in the electrical manipulation of a single nuclear spin, crucial for the future of quantum information processing. It highlights the development of a molecular transistor capable of writing quantum information onto a nuclear spin using only an electric field, enabling rapid electronic read-out of the quantum state. By leveraging single-molecule magnets, the work paves the way for high-speed manipulation of individual nuclear spins within confined spaces, potentially revolutionizing molecular quantum electronics and opening new research avenues.